Nuclear fallout


Nuclear fallout
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Fallout is the residual radioactively charged material propelled into the upper atmosphere following a nuclear blast, so called because it "falls out" of the sky after the explosion and shock wave have passed. It commonly refers to the radioactive dust and ash created when a nuclear weapon explodes. This radioactive dust, consisting of materiel either directly vaporized by a nuclear blast or charged by exposure, is a highly dangerous kind of radioactive contamination. It can lead to the contamination of aquifers and devastate the effected ecosystem years after the initial exposure.

Contents

Types

There are many types of fallout, ranging from the global type to the more area-restricted types of fallout.

Worldwide

After an air burst, fission products, un-fissioned nuclear material, and weapon residues vaporized by the heat of the fireball condense into a fine suspension of small particles 10 nm to 20 µm in diameter. These particles may be quickly drawn up into the stratosphere, particularly if the explosive yield exceeds 10 kt.

Atmospheric nuclear weapon tests almost doubled the concentration of radioactive 14C in the Northern Hemisphere, before levels slowly declined following the Partial Test Ban Treaty.

Initially little was known about the dispersion of nuclear fallout on a global scale. The AEC assumed that fallout would be dispersed evenly across the globe by atmospheric winds and gradually settle to the Earth's surface after weeks, months, and even years as worldwide fallout. Nuclear products were deposited in the Northern Hemisphere becoming "far more dangerous than they had originally been estimated[citation needed]."

The radio-biological hazard of worldwide fallout is essentially a long-term one because of the potential accumulation of long-lived radioisotopes (such as strontium-90 and caesium-137) in the body as a result of ingestion of foods containing the radioactive materials. This hazard is less pertinent than local fallout, which is of much greater immediate operational concern.

Local

In a land or water surface burst, heat vaporizes large amounts of earth or water, which is drawn up into the radioactive cloud. This material becomes radioactive when it condenses with fission products and other radiocontaminants that have become neutron-activated. Most of the isotopes in the table below mostly decay into the isotopes that many people are more familiar with. Some radiation would taint large amounts of land and drinking water causing formal mutations throughout animal and human life.

The roughly 280 mile long fallout plume from 15 Mt shot Castle Bravo, ca. 1954
Table (according to T. Imanaka et al.) of the relative abilities of isotopes to form solids
Isotope 91Sr 92Sr 95Zr 99Mo 106Ru 131Sb 132Te 134Te 137Cs 140Ba 141La 144Ce
Refractory index 0.2 1.0 1.0 1.0 0.0 0.1 0.0 0.0 0.0 0.3 0.7 1.0
Per capita thyroid doses in the continental United States resulting from all exposure routes from all atmospheric nuclear tests conducted at the Nevada Test Site from 1951-1962.

A surface burst generates large amounts of particulate matter, composed of particles from less than 100 nm to several millimeters in diameter—in addition to very fine particles that contribute to worldwide fallout. The larger particles spill out of the stem and cascade down the outside of the fireball in a downdraft even as the cloud rises, so fallout begins to arrive near ground zero within an hour. More than half the total bomb debris lands on the ground within about 24 hours as local fallout. Chemical properties of the elements in the fallout control the rate at which they are deposited on the ground. Less volatile elements deposit first.

Severe local fallout contamination can extend far beyond the blast and thermal effects, particularly in the case of high yield surface detonations. The ground track of fallout from an explosion depends on the weather situation from the time of detonation onwards. In stronger winds, fallout travels faster but takes the same time to descend, so although it covers a larger path, it is more spread out or diluted. So the width of the fallout pattern for any given dose rate is reduced where the downwind distance is increased by higher winds. The total amount of activity deposited up to any given time is the same irrespective of the wind pattern, so overall casualty figures from fallout are generally independent of winds. But thunderstorms can bring down activity as rain more rapidly than dry fallout, particularly if the mushroom cloud is low enough to be below ("washout"), or mixed with ("rainout"), the thunderstorm.

Whenever individuals remain in a radiologically contaminated area, such contamination leads to an immediate external radiation exposure as well as a possible later internal hazard from inhalation and ingestion of radiocontaminants, such as the rather short-lived iodine-131, which is accumulated in the thyroid.

Factors affecting fallout

Location

There are two main considerations for the location of an explosion: height and surface composition. A nuclear weapon detonated in the air, called an air burst, produces less fallout than a comparable explosion near the ground.

In case of water surface bursts, the particles tend to be rather lighter and smaller, producing less local fallout but extending over a greater area. The particles contain mostly sea salts with some water; these can have a cloud seeding effect causing local rainout and areas of high local fallout. Fallout from a seawater burst is difficult to remove once it has soaked into porous surfaces because the fission products are present as metallic ions that chemically bond to many surfaces. Water and detergent washing effectively removes less than 50% of this chemically bonded activity from concrete or steel. Complete decontamination requires aggressive treatment like sandblasting, or acidic treatment. After the Crossroads underwater test, it was found that wet fallout must be immediately removed from ships by continuous water washdown (such as from the fire sprinkler system on the decks).

Parts of the sea bottom may become fallout. After the Castle Bravo test, white dust – contaminated calcium oxide particles originating from pulverized and calcined corals – fell for several hours, causing beta burns and radiation exposition to the inhabitants of the nearby atolls and the crew of the Daigo Fukuryū Maru fishing boat. The scientists called the fallout Bikini snow.

For subsurface bursts, there is an additional phenomenon present called "base surge". The base surge is a cloud that rolls outward from the bottom of the subsiding column, which is caused by an excessive density of dust or water droplets in the air. For underwater bursts, the visible surge is, in effect, a cloud of liquid (usually water) droplets with the property of flowing almost as if it were a homogeneous fluid. After the water evaporates, an invisible base surge of small radioactive particles may persist.

For subsurface land bursts, the surge is made up of small solid particles, but it still behaves like a fluid. A soil earth medium favors base surge formation in an underground burst. Although the base surge typically contains only about 10% of the total bomb debris in a subsurface burst, it can create larger radiation doses than fallout near the detonation, because it arrives sooner than fallout, before much radioactive decay has occurred.

Meteorological

Comparison of fallout gamma dose and dose rate contours for a 1 Mt fission land surface burst, based on DELFIC calculations. Because of radioactive decay, the dose rate contours contract after fallout has arrived, but dose contours continue to grow

Meteorological conditions greatly influence fallout, particularly local fallout. Atmospheric winds are able to bring fallout over large areas. For example, as a result of a Castle Bravo surface burst of a 15 Mt thermonuclear device at Bikini Atoll on March 1, 1954, a roughly cigar-shaped area of the Pacific extending over 500 km downwind and varying in width to a maximum of 100 km was severely contaminated. There are three very different versions of the fallout pattern from this test, because the fallout was only measured on a small number of widely spaced Pacific Atolls. The two alternative versions both ascribe the high radiation levels at north Rongelap to a downwind hotspot caused by the large amount of radioactivity carried on fallout particles of about 50-100 micrometres size.[1]

After Bravo, it was discovered that fallout landing on the ocean disperses in the top water layer (above the thermocline at 100 m depth), and the land equivalent dose rate can be calculated by multiplying the ocean dose rate at two days after burst by a factor of about 530. In other 1954 tests, including Yankee and Nectar, hotspots were mapped out by ships with submersible probes, and similar hotspots occurred in 1956 tests such as Zuni and Tewa.[2] However, the major U.S. 'DELFIC' (Defence Land Fallout Interpretive Code) computer calculations use the natural size distributions of particles in soil instead of the afterwind sweep-up spectrum, and this results in more straightforward fallout patterns lacking the downwind hotspot.

Snow and rain, especially if they come from considerable heights, accelerate local fallout. Under special meteorological conditions, such as a local rain shower that originates above the radioactive cloud, limited areas of heavy contamination just downwind of a nuclear blast may be formed.

Effects

A wide range of biological changes may follow the irradiation of animals. These vary from rapid death following high doses of penetrating whole-body radiation, to essentially normal lives for a variable period of time until the development of delayed radiation effects, in a portion of the exposed population, following low dose exposures.

The unit of actual exposure is the röntgen, defined in ionisations per unit volume of air. All ionisation based instruments (including geiger counters and ionisation chambers) measure exposure. However, effects depend on the energy per unit mass, not the exposure measured in air. A deposit of 1 joule per kilogram has the unit of 1 gray (Gy). For 1 MeV energy gamma rays, an exposure of 1 röntgen in air produces a dose of about 0.01 gray (1 centigray, cGy) in water or surface tissue. Because of shielding by the tissue surrounding the bones, the bone marrow only receives about 0.67 cGy when the air exposure is 1 röntgen and the surface skin dose is 1 cGy. Some lower values reported for the amount of radiation that would kill 50% of personnel (the LD50) refer to bone marrow dose, which is only 67% of the air dose.

Short term

Fallout shelter sign on a building in New York City.

The dose that would be lethal to 50% of a population is a common parameter used to compare the effects of various fallout types or circumstances. Usually, the term is defined for a specific time, and limited to studies of acute lethality. The common time periods used are 30 days or less for most small laboratory animals and to 60 days for large animals and humans. The LD50 figure assumes that the individuals did not receive other injuries or medical treatment.

In the 1950s, the LD50 for gamma rays was set at 3.5 Gy, while under more dire conditions of war (a bad diet, little medical care, poor nursing) the LD50 was 2.5 Gy (250 rad). There have been few documented cases of survival beyond 6 Gy. One person at Chernobyl survived a dose of more than 10 Gy, but many of the persons exposed there were not uniformly exposed over their entire body. If a person is exposed in a non-homogeneous manner than a given dose (averaged over the entire body) is less likely to be lethal. For instance, if a person gets a hand/low arm dose of 100 Gy, which gives them an overall dose of 4 Gy, they are more likely to survive than a person who gets a 4 Gy dose over their entire body. A hand dose of 10 Gy or more would likely result in loss of the hand. A British industrial radiographer who got a lifetime hand dose of 100 Gy lost his hand because of radiation dermatitis[citation needed]. Most people become ill after an exposure to 1 Gy or more. The fetuses of pregnant women are often more vulnerable to radiation and may miscarry, especially in the first trimester.

One hour after a surface burst, the radiation from fallout in the crater region is 30 grays per hour (Gy/h)[clarification needed]. Civilian dose rates in peacetime range from 30 to 100 µGy per year.

Fallout radiation decays exponentially relatively quickly with time. Most areas become fairly safe for travel and decontamination after three to five weeks.

For yields of up to 10 kt, prompt radiation is the dominant producer of casualties on the battlefield. Humans receiving an acute incapacitating dose (30 Gy) have their performance degraded almost immediately and become ineffective within several hours. However, they do not die until five to six days after exposure, assuming they do not receive any other injuries. Individuals receiving less than a total of 1.5 Gy are not incapacitated. People receiving doses greater than 1.5 Gy become disabled, and some eventually die.

A dose of 5.3 Gy to 8.3 Gy is considered lethal but not immediately incapacitating. Personnel exposed to this amount of radiation have their performance degraded in two to three hours, depending on how physically demanding the tasks they must perform are, and remain in this disabled state at least two days. However, at that point they experience a recovery period and can perform non-demanding tasks for about six days, after which they relapse for about four weeks. At this time they begin exhibiting symptoms of radiation poisoning of sufficient severity to render them totally ineffective. Death follows at approximately six weeks after exposure, although outcomes may vary.

Long term

Late or delayed effects of radiation occur following a wide range of doses and dose rates. Delayed effects may appear months to years after irradiation and include a wide variety of effects involving almost all tissues or organs. Some of the possible delayed consequences of radiation injury are life shortening, carcinogenesis, cataract formation, chronic radiodermatitis, decreased fertility, and genetic mutations.[3]

Tactical military considerations

Comparison of predicted fallout "hotline" with test results in the 3.53 Mt 15% fission Zuni test at Bikini in 1956. The predictions were made under simulated tactical nuclear war conditions aboard ship by Edward A. Schuert.

In many cases, blast injuries and thermal burns from nuclear weapons will far outnumber radiation injuries. However, radiation effects are considerably more complex and varied than are blast or thermal effects and are subject to considerable misunderstanding.

The closer to ground an atomic bomb is detonated, the more dust and debris is thrown into the air, resulting in greater amounts of local fallout. From a tactical standpoint, this has the disadvantage of hindering any occupation/invading efforts until the fallout clears, but more directly, the impact with the ground severely limits the destructive force of the bomb. For these reasons, ground bursts are not usually considered tactically advantageous, with the exception of hardened underground targets such as missile silos or command centers; however "salting" enemy territory with a fallout-heavy atomic burst or a salted bomb can be used to deny ill-equipped civilians and military personnel access to a contaminated area.

Fallout protection

During the Cold War, the governments of the U.S., the USSR, Great Britain, and China attempted to educate their citizens about surviving a nuclear attack by providing procedures on minimizing short-term exposure to fallout. In the U.S. and China, this effort became known as Civil Defense.

Nuclear reactor accident

Fallout can also refer to nuclear accidents, although a nuclear reactor does not explode like a nuclear weapon. The isotopic signature of bomb fallout is very different from the fallout from a serious power reactor accident (such as Chernobyl or Fukushima). The key differences are in volatility and half-life.

Volatility

The boiling point of an element (or its compounds) is able to control the percentage of that element a power reactor accident releases. In addition, the ability of an element to form a solid controls the rate it is deposited on the ground after having been injected into the atmosphere by a nuclear detonation or accident.

Half-life

A large amount of short-lived isotopes such as 97Zr are present in bomb fallout. This isotope and other short-lived isotopes are constantly generated in a power reactor, but because the criticality occurs over a long length of time, the majority of these short lived isotopes decay before they can be released.

Below is shown a comparison of the calculated gamma dose rates in open air from the fallout of a fission bomb and of the Chernobyl release. It is clear that average half-life of the Chernobyl release is longer than that for the bomb fallout.

See also

References

Footnotes

  1. ^ [1]
  2. ^ [2]
  3. ^ Simon, Steven L.; Bouville, André; Land, Charles E. (2006), Fallout from Nuclear Weapons Tests and Cancer Risks, 94, American Scientist, pp. 48–57 

General references

  • Glasstone, Samuel and Dolan, Philip J., The Effects of Nuclear Weapons (third edition), U.S. Government Printing Office, 1977. (Available Online)
  • NATO Handbook on the Medical Aspects of NBC Defensive Operations (Part I - Nuclear), Departments of the Army, Navy, and Air Force, Washington, D.C., 1996, (Available Online)
  • Smyth, H. DeW., Atomic Energy for Military Purposes, Princeton University Press, 1945. (Smyth Report)
  • The Effects of Nuclear War in America, Office of Technology Assessment (May 1979) (Available Online)
  • T. Imanaka, S. Fukutani, M. Yamamoto, A. Sakaguchi and M. Hoshi, J. Radiation Research, 2006, 47, Suppl A121-A127.
  • Sheldon Novick, The Careless Atom, (Boston MA: Houghton Mifflin Co., 1969), p. 98
  • Fallout game

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